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Emerging Study on Lead‐Free Hybrid Double Perovskite (CH<sub>3</sub>NH<sub>3</sub>)<sub>2</sub>AgInBr<sub>6</sub>: Potential Material for Energy Conversion between Heat and Electricity

Upasana Rani, Peeyush Kumar Kamlesh, Rohit Agrawal, Akash Shukla, Ajay Singh Verma

2022Energy Technology78 citationsDOI

Abstract

Minimal cost, huge area, high throughput, high performance of photovoltaic panels, prolonged lifespan, and less toxicity are vital aspects when transitioning photovoltaic technology from lab‐scale production to industrial implementations. A new class of materials typically known as hybrid halide double perovskites (HHDPs) has emerged as a possible alternative for the replacement of toxic lead in crystal lattice for realizing lead‐free, stable, and high‐performance perovskite solar cells (PSCs). An ab initio analysis of (MA) 2 AgInBr 6 HHDP via the WIEN2K code is conducted. It is found that this material has a direct bandgap of 3.85 eV having excellent optical properties in the UV region. The calculated thermodynamic parameters confirm its thermal stability at different temperatures and pressure. Its figure of merit is more than unity at room temperature as well as higher temperature ranges, so this material will be useful in thermoelectric (TE) devices as a TE material.

Topics & Concepts

Materials sciencePhotovoltaic systemFigure of meritBand gapWIEN2kPerovskite (structure)Thermal stabilityOptoelectronicsHalideEnergy conversion efficiencyThermoelectric effectDensity functional theoryThermodynamicsChemistryInorganic chemistryElectrical engineeringLocal-density approximationComputational chemistryCrystallographyPhysicsOrganic chemistryEngineeringPerovskite Materials and ApplicationsSolid-state spectroscopy and crystallographyChalcogenide Semiconductor Thin Films