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Manipulating Two-Photon-Absorption of Cavity Polaritons by Entangled Light

Bing Gu, Shaul Mukamel

2020The Journal of Physical Chemistry Letters34 citationsDOI

Abstract

We demonstrate that two-photon excitations to bipolariton states created by placing several molecules in an optical cavity can be manipulated by quantum light. Entangled photons can access classically dark bipolariton states by modifying the quantum interferences of two-photon transition pathways involving different single-polariton intermediate states and time-ordering of the two photon beams.

Topics & Concepts

PolaritonPhotonPhysicsQuantum opticsAbsorption (acoustics)Photon entanglementQuantumOptoelectronicsQuantum mechanicsAtomic physicsQuantum entanglementOpticsStrong Light-Matter InteractionsQuantum Information and CryptographyPlasmonic and Surface Plasmon Research
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