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A conductive rubber with self‐healing ability enabled by metal‐ligand coordination

Jianxiang Xiong, Zhou Gong, Jianping Ding, Yukun Chen

2021Polymers for Advanced Technologies15 citationsDOI

Abstract

Abstract At present, flexible conductive materials have been widely noticed. However, developing electronic materials with both good mechanical and electrical self‐healing abilities remains both a great challenge and an exciting goal. Herein, we prepared a commercial nitrile butadiene rubber (NBR) with electrical healing capability based on constructing Fe(III) coordination and CNT networks. With 3 phr (parts per hundreds of rubber) CNT, the tensile strength and the elongation at break of rubber composite reached 1.1 MPa and 300%, respectively. After healing at 80°C for 9 hours, the recovery efficiency of rubber composite achieved 90%. After adding 5 phr CNT, the conductivity can reach 0.077 S/m, and the electrical conductivity was 0.076 S/m after self‐healing. Such material can maintain resistance change within 5 times at high strain (100%), so it is applicable in the field of strain sensor.

Topics & Concepts

Materials scienceNatural rubberComposite materialUltimate tensile strengthElectrical conductorComposite numberElongationSelf-healingMetalElectrical resistivity and conductivityMetallurgyElectrical engineeringMedicinePathologyAlternative medicineEngineeringAdvanced Sensor and Energy Harvesting MaterialsConducting polymers and applicationsPolymer composites and self-healing
A conductive rubber with self‐healing ability enabled by metal‐ligand coordination | Litcius