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Engendering persistent organic room temperature phosphorescence by trace ingredient incorporation

Bingbing Ding, Liangwei Ma, Zizhao Huang, Xiang Ma, He Tian

2021Science Advances231 citationsDOIOpen Access PDF

Abstract

Pure organic persistent room temperature phosphorescence (RTP) has shown great potential in information encryption, optoelectronic devices, and bio-applications. However, trace impurities are generated in synthesis, causing unpredictable effects on the luminescence properties. Here, an impurity is isolated from a pure organic RTP system and structurally characterized that caused an unusual ultralong RTP in matrix even at 0.01 mole percent content. Inspired by this effect, a series of compounds are screened out to form the bicomponent RTP system by the trace ingredient incorporation method. The RTP quantum yields reach as high as 74.2%, and the lifetimes reach up to 430 ms. Flexible application of trace ingredients to construct RTP materials has become an eye-catching strategy with high efficiency, economy, and potential for applications as well as easy preparation.

Topics & Concepts

PhosphorescenceTRACE (psycholinguistics)IngredientPersistent luminescenceMaterials scienceActive ingredientNanotechnologyEnvironmental chemistryChemistryOptoelectronicsLuminescenceFluorescenceOpticsBioinformaticsPhysicsFood sciencePhilosophyThermoluminescenceBiologyLinguisticsLuminescence and Fluorescent MaterialsOrganic Light-Emitting Diodes ResearchMolecular Sensors and Ion Detection
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