Revealing Excitonic and Electron-Hole Plasma States in Stimulated Emission of Single <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline" overflow="scroll"><mml:msub><mml:mrow><mml:mi>Cs</mml:mi><mml:mi>Pb</mml:mi><mml:mi>Br</mml:mi></mml:mrow><mml:mn>3</mml:mn></mml:msub></mml:math> Nanowires at Room Temperature
Mai He, Ying Jiang, Qingbo Liu, Ziyu Luo, Chenxing Ouyang, Xiaoxia Wang, Weihao Zheng, Kai Braun, Alfred J. Meixner, Tingge Gao, Xiao Wang, Anlian Pan
Abstract
Nanostructured lead halide perovskites have received extensive attention due to their potential applications in integrated photonics. Despite many successful realizations of nanoscale coherent-light sources from lead halide perovskites, the role and interplay between excitonic and electron-hole plasma (EHP) states in the stimulated-emission process are not demonstrated yet. In this work, the carrier behavior and dynamics of the stimulated emission in ${\mathrm{Cs}\mathrm{Pb}\mathrm{Br}}_{3}$ single nanowires are studied with a streak camera under power-dependent one-photon and two-photon excitation at room temperature. A redshift of the lasing gain profile with increasing excitation fluence is observed, suggesting the transition from the excitonic state to EHP state that is responsible for the lasing. Whereas, a blueshift of the gain profile with time decay represents the opposite direction of the former process. Moreover, the individual lasing modes show a blueshift as excitation fluence increases and a redshift as time elapses, due to the carrier-density dependence of the refractive index. This study could provide a comprehensive and deeper understanding of the carrier-density-driven stimulated-emission dynamics in lead halide nanowires and extend their applications in integrated photonics.