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Mn-Doped black phosphorene for ultrasensitive hydrogen sulfide detection: periodic DFT calculations

Mahdi Ghadiri, Mohammad Ghashghaee, Mehdi Ghambarian

2020Physical Chemistry Chemical Physics46 citationsDOI

Abstract

S nanosensor in terms of both electric conductance (3747) and work function (11 times more sensitive) through Mn doping. The new sensor was also highly selective, with a sensitivity ratio of at least 52.6 with respect to the air components. The recovery time of the Mn-doped material (2.7 s at ambient temperature) was more promising than that of BP from a practical point of view. More discussion of the material is presented with the electronic properties, frontier molecular orbitals, and density of states at rest and under operating conditions.

Topics & Concepts

PhosphoreneBlack phosphorusMonolayerDopingMaterials scienceConductanceNanosensorWork functionHydrogen sulfideNanotechnologyChemical physicsInorganic chemistryChemistryOptoelectronicsCondensed matter physicsPhysicsLayer (electronics)MetallurgySulfur2D Materials and ApplicationsPerovskite Materials and ApplicationsMXene and MAX Phase Materials
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