Litcius/Paper detail

Electron–Electron Dipolar Interaction Poses a Challenge to the Radical Pair Mechanism of Magnetoreception

Nathan S. Babcock, Daniel R. Kattnig

2020The Journal of Physical Chemistry Letters58 citationsDOIOpen Access PDF

Abstract

hyperfine interactions. Prior studies have often neglected the electron-electron dipolar (EED) coupling from this hypothesis. We show that EED interactions suppress the anisotropic response to the geomagnetic field by the radical pair mechanism in cryptochrome and that this attenuation is unlikely to be mitigated by mutual cancellation of the EED and electronic exchange coupling, as previously suggested. We then demonstrate that this limitation may be overcome by extending the conventional model to include a third, nonreacting radical. We predict that hyperfine effects could work in concert with three-radical dipolar interactions to tailor a superior magnetic response, thereby providing a new principle for magnetosensitivity with applications for sensing, navigation, and the assessment of biological magnetic field effects.

Topics & Concepts

MagnetoreceptionCryptochromeHyperfine structureElectron transferElectronEarth's magnetic fieldMagnetic dipole–dipole interactionMagnetic fieldChemical physicsPhysicsDipoleChemistryPhotochemistryAtomic physicsQuantum mechanicsBiochemistryCircadian clockGeneElectromagnetic Fields and Biological EffectsPhotoreceptor and optogenetics researchAtomic and Subatomic Physics Research