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Mild and Regioselective Three‐component Heteroarylation‐Nitration of Alkenes with Imidazo[1,2‐<i>a</i>]pyridines and <i>tert</i>‐Butyl Nitrite

Jie Zhang, Shentong Xie, Ping Liu, Peipei Sun

2020Advanced Synthesis & Catalysis29 citationsDOI

Abstract

Abstract An efficient and regioselective three‐component heteroarylation‐nitration of alkenes with imidazo[1,2‐ a ]pyridines and tert ‐butyl nitrite has been developed. The process tolerants a variety of functional groups under mild conditions in the absence of catalysts and additives to give nitro functionalized imidazo[1,2‐ a ]pyridine derivatives in moderate to good yields. The reaction is also applicable for some other aza‐heterocycles. magnified image

Topics & Concepts

NitrationRegioselectivityChemistryNitritePyridineNitroCatalysisComponent (thermodynamics)Organic chemistryMedicinal chemistryCombinatorial chemistryNitrateAlkylThermodynamicsPhysicsCatalytic C–H Functionalization MethodsPhenothiazines and Benzothiazines Synthesis and ActivitiesSynthesis and Catalytic Reactions
Mild and Regioselective Three‐component Heteroarylation‐Nitration of Alkenes with Imidazo[1,2‐<i>a</i>]pyridines and <i>tert</i>‐Butyl Nitrite | Litcius