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Combining photocontrolled-cationic and anionic-group-transfer polymerizations using a universal mediator: enabling access to two- and three-mechanism block copolymers

Brandon Hosford, William Ramos, Jessica R. Lamb

2024Chemical Science11 citationsDOIOpen Access PDF

Abstract

three different mechanisms without any end-group modification steps. The development of this simple, sequential synthesis using a universal mediator approach opens up new possibilities by providing facile access to diverse block copolymers of vinyl ethers, thiiranes, and acrylamides.

Topics & Concepts

Cationic polymerizationCopolymerVinyl etherLiving cationic polymerizationThiiranePolymer chemistryAnionic addition polymerizationChemistryBlock (permutation group theory)Group (periodic table)PolymerizationEtherMaterials sciencePolymerOrganic chemistryMathematicsGeometryRing (chemistry)Advanced Polymer Synthesis and CharacterizationPhotopolymerization techniques and applicationsSynthetic Organic Chemistry Methods