Yb:GdScO<sub>3</sub> crystal for efficient ultrashort pulse lasers
Yuhang Zhang, Shanming Li, Xiaoqiang Du, Jie Guo, Qiaorui Gong, Siliang Tao, Peixiong Zhang, Qiannan Fang, Shilie Pan, Chengchun Zhao, Xiaoyan Liang, Hang Yin
Abstract
We present, to the best of our knowledge, the first demonstration of thermal, optical, and laser properties of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mi mathvariant="normal">Y</mml:mi> <mml:mi mathvariant="normal">b</mml:mi> </mml:mrow> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mo>:</mml:mo> </mml:mrow> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:msub> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mi mathvariant="normal">G</mml:mi> <mml:mi mathvariant="normal">d</mml:mi> <mml:mi mathvariant="normal">S</mml:mi> <mml:mi mathvariant="normal">c</mml:mi> <mml:mi mathvariant="normal">O</mml:mi> </mml:mrow> <mml:mn>3</mml:mn> </mml:msub> </mml:mrow> </mml:math> for potentially efficient ultrashort pulse lasers. The stimulated emission cross section at 1025 nm (E//c) is <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mn>0.46</mml:mn> </mml:mrow> <mml:mo>×</mml:mo> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:msup> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mn>10</mml:mn> </mml:mrow> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mo>−</mml:mo> <mml:mn>20</mml:mn> </mml:mrow> </mml:msup> </mml:mrow> <mml:mspace width="thickmathspace"/> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:msup> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mi mathvariant="normal">c</mml:mi> <mml:mi mathvariant="normal">m</mml:mi> </mml:mrow> <mml:mn>2</mml:mn> </mml:msup> </mml:mrow> </mml:math> with the emission band width of 85 nm, even broader than the well-known <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mi mathvariant="normal">Y</mml:mi> <mml:mi mathvariant="normal">b</mml:mi> </mml:mrow> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mo>:</mml:mo> </mml:mrow> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:msub> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mi mathvariant="normal">C</mml:mi> <mml:mi mathvariant="normal">a</mml:mi> <mml:mi mathvariant="normal">G</mml:mi> <mml:mi mathvariant="normal">d</mml:mi> <mml:mi mathvariant="normal">A</mml:mi> <mml:mi mathvariant="normal">l</mml:mi> <mml:mi mathvariant="normal">O</mml:mi> </mml:mrow> <mml:mn>4</mml:mn> </mml:msub> </mml:mrow> </mml:math> . It has quite a high thermal conductivity of <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mn>5.54</mml:mn> </mml:mrow> <mml:mspace width="thickmathspace"/> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mi mathvariant="normal">W</mml:mi> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mo>/</mml:mo> </mml:mrow> </mml:mrow> <mml:mo stretchy="false">(</mml:mo> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mi mathvariant="normal">m</mml:mi> <mml:mo>⋅</mml:mo> <mml:mi mathvariant="normal">K</mml:mi> </mml:mrow> <mml:mo stretchy="false">)</mml:mo> </mml:math> at 50°C, comparable with Yb:YAG. In the continuous-wave regime, the maximum output power of 13.45 W at 1063.9 nm was generated with the optical-to-optical efficiency of 63.3%. These results suggest that the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mi mathvariant="normal">Y</mml:mi> <mml:mi mathvariant="normal">b</mml:mi> </mml:mrow> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mo>:</mml:mo> </mml:mrow> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:msub> <mml:mrow class="MJX-TeXAtom-ORD"> <mml:mi mathvariant="normal">G</mml:mi> <mml:mi mathvariant="normal">d</mml:mi> <mml:mi mathvariant="normal">S</mml:mi> <mml:mi mathvariant="normal">c</mml:mi> <mml:mi mathvariant="normal">O</mml:mi> </mml:mrow> <mml:mn>3</mml:mn> </mml:msub> </mml:mrow> </mml:math> crystal is a promising candidate for ultrashort pulse lasers.