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Effective modeling of open quantum systems by low-rank discretization of structured environments

H. Takahashi, Raffaele Borrelli

2024The Journal of Chemical Physics11 citationsDOI

Abstract

The accurate description of the interaction of a quantum system with its environment is a challenging problem ubiquitous across all areas of physics and lies at the foundation of quantum mechanics theory. Here, we pioneer a new strategy to create discrete low-rank models of the system-environment interaction, by exploiting the frequency and time domain information encoded in the fluctuation-dissipation relation connecting the system-bath correlation function and the spectral density. We demonstrate the effectiveness of our methodology by combining it with tensor-network methodologies and simulating the quantum dynamics of complex excitonic systems in a highly structured bosonic environment. The new modeling framework sets the basis for a leap in the analysis of open quantum systems, providing controlled accuracy at significantly reduced computational costs, with benefits in all connected research areas.

Topics & Concepts

Computer scienceDiscretizationQuantumTensor (intrinsic definition)Rank (graph theory)Relation (database)Statistical physicsTheoretical computer scienceDomain (mathematical analysis)Function (biology)Complex systemQuantum systemPhysicsQuantum mechanicsMathematicsArtificial intelligenceData miningEvolutionary biologyBiologyMathematical analysisCombinatoricsPure mathematicsTensor decomposition and applicationsQuantum many-body systemsSpectroscopy and Quantum Chemical Studies
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