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Thin-film solid-phase microextraction of pesticides from cereal samples using electrospun polyvinyl alcohol/modified chitosan/porous organic framework nanofibers

Mahshid Majd, Marziye Gholami, Anna Fathi, Roya Sedghi, Saeed Nojavan

2024Food Chemistry20 citationsDOIOpen Access PDF

Abstract

In this study, a coating of electrospun polyvinyl alcohol/modified chitosan/hydroxy-containing porous organic framework (PVA/MCS/HC-POF) was fabricated and applied as a novel sorbent for thin-film solid-phase microextraction of pesticides from cereal samples, followed by HPLC-UV. The successful fabrication of PVA/MCS/HC-POF was confirmed through characterization tests. The functional group of MCS and a large number of hydroxyl groups on the HC-POF structure contributed to the co-extraction of pesticides. Under the optimum conditions, the calibration plots were linear within the range of 5.0–800 ng mL −1 (r 2 ≥ 0.978), and the limits of detection were obtained below 4.0 ng mL −1 . The method's precision was investigated through intra-day, inter-day, and film-to-film RSD (%) measurements, all of which were less than 6.5 %, 8.2 %, and 10.0 %, respectively. Furthermore, satisfactory recoveries ranging from 63.3 % to 79.0 % were obtained. Accordingly, the proposed method can be considered a suitable alternative for measuring trace amounts of pesticides in cereal samples.

Topics & Concepts

Polyvinyl alcoholSolid-phase microextractionNanofiberSorbentChitosanMaterials scienceChromatographyPorosityDetection limitExtraction (chemistry)ChemistryNanotechnologyMass spectrometryGas chromatography–mass spectrometryComposite materialOrganic chemistryAdsorptionAnalytical chemistry methods developmentElectrochemical sensors and biosensorsElectrochemical Analysis and Applications
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