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Coherent spin-control of <i>S</i> = 1 vanadium and molybdenum complexes

Daniel W. Laorenza, Kathleen R. Mullin, Leah R. Weiss, Sam L. Bayliss, Pratiti Deb, D. D. Awschalom, James M. Rondinelli, Danna E. Freedman

2024Chemical Science12 citationsDOIOpen Access PDF

Abstract

, complexes may not be suitable candidate optically addressable qubit systems due to their low energy spin-singlet states. By understanding the failures and successes of these systems, we outline additional design features for optically addressable V- or Mo-based molecules to expand the library of tailor-made quantum sensors.

Topics & Concepts

MolybdenumVanadiumSpin (aerodynamics)Materials scienceChemistryInorganic chemistryPhysicsThermodynamicsMagnetism in coordination complexesDiamond and Carbon-based Materials ResearchOrganic and Molecular Conductors Research
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