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Ultrahigh-Q Lead Halide Perovskite Microlasers

Haijun Tang, Yuhan Wang, Yimu Chen, Kaiyang Wang, Xianxiong He, Can Huang, Shumin Xiao, Shaohua Yu, Qinghai Song

2023Nano Letters29 citationsDOI

Abstract

Lead halide perovskites have been promising platforms for micro- and nanolasers. However, the fragile nature of perovskites poses an extreme challenge to engineering a cavity boundary and achieving high-quality (Q) modes, severely hindering their practical applications. Here, we combine an etchless bound state in the continuum (BIC) and a chemically synthesized single-crystalline CsPbBr 3 microplate to demonstrate on-chip integrated perovskite microlasers with ultrahigh Q factors. By pattering polymer microdisks on CsPbBr 3 microplates, we show that record high-Q BIC modes can be formed by destructive interference between different in-plane radiation from whispering gallery modes. Consequently, a record high Q-factor of 1.04 × 10 5 was achieved in our experiment. The high repeatability and high controllability of such ultrahigh Q BIC microlasers have also been experimentally confirmed. This research provides a new paradigm for perovskite nanophotonics.

Topics & Concepts

HalidePerovskite (structure)Materials scienceNanophotonicsResonatorOptoelectronicsControllabilityWhispering-gallery waveQ factorPhotonicsNanotechnologyOpticsCrystallographyPhysicsChemistryInorganic chemistryMathematicsApplied mathematicsPerovskite Materials and ApplicationsPhotorefractive and Nonlinear OpticsPhotonic and Optical Devices
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