Litcius/Paper detail

Attosecond-Scale Streaking Methods for Strong-Field Ionization by Tailored Fields

Nicolas Eicke, Simon Brennecke, Manfred Lein

2020Physical Review Letters38 citationsDOI

Abstract

Streaking with a weak probe field is applied to ionization in a two-dimensional strong field tailored to mimic linear polarization, but without disturbance by recollision or intracycle interference. This facilitates the observation of electron-momentum-resolved times of ionization with few-attosecond precision, as demonstrated by simulations for a model helium atom. Aligning the probe field along the ionizing field provides meaningful ionization times in agreement with the attoclock concept that ionization at maximum field corresponds to the peak of the momentum distribution, which is shifted due to the Coulomb force on the outgoing electron. In contrast, this attoclock shift is invisible in orthogonal streaking. Even without a probe field, streaking happens naturally along the laser propagation direction due to the laser magnetic field. As with an orthogonal probe field, the attoclock shift is not accessible by the magnetic-field scheme. For a polar molecule, the attoclock shift depends on orientation, but this does not imply an orientation dependence in ionization time.

Topics & Concepts

StreakingAttosecondPhysicsIonizationAtomic physicsElectronDouble ionizationField (mathematics)Field desorptionMomentum (technical analysis)Electric fieldMagnetic fieldLaserOpticsUltrashort pulseIonQuantum mechanicsPure mathematicsEconomicsMathematicsFinanceLaser-Matter Interactions and ApplicationsLaser-Plasma Interactions and DiagnosticsAtomic and Molecular Physics