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Toward Smart SiC Self-Powered Deep Ultraviolet Photodetectors

Siying Gao, Lei Ge, Guangcan Wang, Junchen Wan, Zixu Sa, Pengsheng Li, Zeqi Zang, Mingsheng Xu, Zaixing Yang

2025The Journal of Physical Chemistry Letters12 citationsDOI

Abstract

The reasonable construction of a heterojunction is promising for wide bandgap semiconductors in smart self-powered deep ultraviolet (DUV) photodetection. In this work, PbI 2 nanosheet (NS) is prepared directly on the wide bandgap semiconductor of a SiC wafer for the success construction of a type-II heterojunction by a simple drop-casting method. Benefiting from the built-in electric field at the heterojunction interface, the as-fabricated SiC type-II heterojunction photodetector exhibits enhanced DUV photoresponse compared to the SiC wafer and PbI 2 NS photodetectors. The as-fabricated SiC type-II heterojunction photodetector further exhibits excellent self-powered photodetection behaviors, including the low dark current of 1.3 × 10 –13 A, high I light / I dark ratio of 1.5 × 10 4, and fast response times of 0.65/0.58 ms. The excellent photodetection performance enables the SiC type-II heterojunction in omnidirectional photodetection and photocommunication. This work paves the way of constructing a SiC heterojunction for high-performance DUV self-powered photodetection.

Topics & Concepts

PhotodetectorUltravioletOptoelectronicsMaterials scienceGa2O3 and related materialsNanowire Synthesis and ApplicationsGaN-based semiconductor devices and materials
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