Litcius/Paper detail

Rational design of elastin-like polypeptide fusion proteins to tune self-assembly and properties of protein vesicles

Yirui Li, Dylan R. Dautel, Mikaela A. Gray, Michael McKenna, Julie A. Champion

2023Journal of Materials Chemistry B24 citationsDOIOpen Access PDF

Abstract

assembly conditions. In order to access a wider range of vesicle diameter and stability profiles, this work investigated how modifiying the hydrophobicity and length of the ELP sequence influenced self-assembly and the final properties of protein vesicles using mCherry as a model globular protein. The results showed that both transition temperature and diameter of protein vesicles were inversely correlated to the ELP guest residue hydrophobicity and the number of ELP pentapeptide repeats. Additionally, sequence manipulation enabled assembly of vesicles with properties not accessible by changes to assembly conditions. For example, introduction of tyrosine at 5 guest residue positions in ELP enabled formation of nanoscale vesicles stable at physiological salt concentration. This work yields design guidelines for modifying the ELP sequence to manipulate protein vesicle transition temperature, size and stability to achieve desired properties for particular biofunctional applications.

Topics & Concepts

ElastinVesicleFusion proteinBiophysicsFusionRational designSelf-assemblyPeptide sequenceSequence (biology)Amino acidChemistryMaterials scienceBiochemistryNanotechnologyRecombinant DNABiologyMembraneGeneLinguisticsPhilosophyGeneticsConnective tissue disorders researchGlycosylation and Glycoproteins ResearchBone and Dental Protein Studies