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Intrinsic defect study on ternary ABX2 diamond-like thermoelectric materials and analysis of the density of energy function

Ying Zhou, Xin Li, Lili Xi, Jiong Yang

2020Journal of Materiomics23 citationsDOIOpen Access PDF

Abstract

The complex intrinsic defects of four ternary diamond-like ABX2 (A: Cu/Ag; B: In; X: Te/Se) compounds are studied by first-principles calculations. The results show that Cu-based compounds are likely to generate acceptor VA defect with p-type, while Ag-based compounds form donor BA with n-type. The reasons are analyzed by the newly introduced density of energy (DOE).

Topics & Concepts

Ternary operationMaterials scienceDiamondAcceptorThermoelectric effectDensity functional theoryThermoelectric materialsThermodynamicsCondensed matter physicsChemical physicsCrystallographyMetallurgyComputational chemistryChemistryProgramming languageComputer sciencePhysicsAdvanced Thermoelectric Materials and DevicesChalcogenide Semiconductor Thin FilmsSemiconductor materials and interfaces