Litcius/Paper detail

Fluxionality of Subnano Clusters Reshapes the Activity Volcano of Electrocatalysis

Zisheng Zhang, Borna Zandkarimi, Julen Munárriz, Claire E. Dickerson, Anastassia N. Alexandrova

2022ChemCatChem26 citationsDOIOpen Access PDF

Abstract

Abstract The Sabatier activity volcano provides intuitive guide for catalyst design, but also imposes fundamental limitations on the composition and maximal activity of catalysts. We show that the ORR activity volcano is shifted and reshaped by the potential‐dependent fluxionality of subnano cluster catalysts. Fluxionality causes the typically under‐binding Ag/Au to gain optimal activity in the cluster form, and surpass Pt/Pd. Furthermore, isomerization of clusters as a function of the potential breaks linear scaling relationships, enabling surpassing the volcano “apex” relative to the bulk. The effect is likely general for fluxional cluster catalysts.

Topics & Concepts

Cluster (spacecraft)CatalysisIsomerizationVolcanoChemistryElectrocatalystChemical physicsScalingComputational chemistryCrystallographyPhysical chemistryGeochemistryGeologyOrganic chemistryMathematicsComputer scienceGeometryElectrodeProgramming languageElectrochemistryElectrocatalysts for Energy ConversionNanocluster Synthesis and ApplicationsMolecular Junctions and Nanostructures