Litcius/Paper detail

Soft X-ray Absorption Spectroscopy for Observing Element-specific Intermolecular Interaction in Solution Chemistry

Masanari Nagasaka, Nobuhiro Kosugi

2021Chemistry Letters25 citationsDOIOpen Access PDF

Abstract

Soft X-ray absorption spectroscopy (XAS) observes element-specific intermolecular interactions of light elements in liquid phase through the core-to-valence excitation. We have newly developed liquid cells and devices with precise photoabsorbance control. We demonstrate here their applications to XAS in transmission measurement with aqueous acetonitrile solutions and XAS in fluorescence-yield measurement with microfluidic systems. Soft X-ray absorption spectroscopy (XAS) can be used to observe element-specific intermolecular interactions of light elements in liquid phase through the core-to-valence excitation. We have newly developed liquid cells and devices with precise photoabsorbance control. We demonstrate here their applications to XAS in transmission measurement with aqueous acetonitrile solutions and XAS in fluorescence-yield measurement with microfluidic systems.

Topics & Concepts

X-ray absorption spectroscopyChemistryAbsorption spectroscopyAcetonitrileIntermolecular forceValence (chemistry)Fluorescence spectroscopySpectroscopyAnalytical Chemistry (journal)Absorption (acoustics)FluorescenceChemical physicsOpticsMoleculeOrganic chemistryPhysicsQuantum mechanicsX-ray Spectroscopy and Fluorescence AnalysisAdvanced X-ray Imaging TechniquesAdvanced MRI Techniques and Applications