Litcius/Paper detail

Towards parameterising atmospheric concentrations of ice-nucleating particles active at moderate supercooling

Claudia Mignani, Jörg Wieder, Michael Sprenger, Zamin A. Kanji, Jan Henneberger, Christine Alewell, Franz Conen

2021Atmospheric chemistry and physics26 citationsDOIOpen Access PDF

Abstract

Abstract. A small fraction of freezing cloud droplets probably initiates much of the precipitation above continents. Only a minute fraction of aerosol particles, so-called ice-nucleating particles (INPs), can trigger initial ice formation at −15 ∘C, at which cloud-top temperatures are frequently associated with snowfall. At a mountaintop site in the Swiss Alps, we found that concentrations of INPs active at −15 ∘C can be parameterised by different functions of coarse (> 2 µm) aerosol particle concentrations, depending on whether an air mass is (a) precipitating, (b) non-precipitating, or (c) carrying a substantial fraction of dust particles while non-precipitating. Consequently, we suggest that a parameterisation at moderate supercooling should consider coarse particles in combination with air mass differentiation.

Topics & Concepts

Ice nucleusSupercoolingAerosolSnowPrecipitationParticle (ecology)Atmospheric sciencesIce crystalsNucleationMass fractionFraction (chemistry)Air mass (solar energy)Environmental scienceChemistryMeteorologyGeologyThermodynamicsChromatographyPhysicsOrganic chemistryOceanographyBoundary layerAtmospheric aerosols and cloudsAtmospheric chemistry and aerosolsFire effects on ecosystems