Modulating intramolecular electron and proton transfer kinetics for promoting carbon dioxide conversion
Yajie Yuan, Yazhen Zhao, Shuai Yang, Sheng Han, Chenbao Lu, Huiping Ji, Tianfu Wang, Changchun Ke, Qing Xu, Jinhui Zhu, Xiaodong Zhuang
Abstract
reduction activity than the pristine iron porphyrin. The maximum CO faradaic efficiency reaches 99.9%, which is the state-of-the-art value among molecular catalysts.
Topics & Concepts
PorphyrinAzuleneIntramolecular forcePhotochemistryProtonDipoleFaraday efficiencyElectron transferChemistryCatalysisViologenCarbon dioxideKineticsMaterials sciencePhysical chemistryOrganic chemistryElectrochemistryElectrodeQuantum mechanicsPhysicsCO2 Reduction Techniques and CatalystsAdvanced battery technologies researchElectrocatalysts for Energy Conversion