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Pinwheel valence bond crystal ground state of the spin-<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mfrac><mml:mn>1</mml:mn><mml:mn>2</mml:mn></mml:mfrac></mml:math> Heisenberg antiferromagnet on the shuriken lattice

Nikita Astrakhantsev, Francesco Ferrari, Nils Niggemann, Tobias Müller, Aishwarya Chauhan, Augustine Kshetrimayum, Pratyay Ghosh, Nicolas Regnault, Ronny Thomale, Johannes Reuther, Titus Neupert, Yasir Iqbal

2021Physical review. B./Physical review. B40 citationsDOIOpen Access PDF

Abstract

Quantum spin models on two-dimensional corner-sharing triangular arrangements, e.g., the kagome lattice, are fertile playgrounds for realizing exotic phases. Following the recent report of a gapless spin liquid in KCu${}_{6}$AlBiO${}_{4}$(SO${}_{4}$)${}_{5}$Cl, wherein the Cu${}^{2+}$ spin-\textonehalf{} ions form a perfect two-dimensional shuriken lattice, the authors employ state-of-the-art quantum many-body approaches to reveal a pinwheel valence-bond-crystal ground state of the isotropic Heisenberg antiferromagnet. This work thus points to the important role of spatial anisotropy in triggering the gapless spin liquid, in contrast to the kagome material herbertsmithite.

Topics & Concepts

Variational Monte CarloQuantum Monte CarloPhysicsValence bond theoryGround stateAntiferromagnetismWave functionValence (chemistry)Quantum mechanicsCondensed matter physicsMonte Carlo methodHubbard modelMoleculeSuperconductivityMolecular orbitalMathematicsStatisticsPhysics of Superconductivity and MagnetismAdvanced Condensed Matter PhysicsQuantum many-body systems
Pinwheel valence bond crystal ground state of the spin-<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mfrac><mml:mn>1</mml:mn><mml:mn>2</mml:mn></mml:mfrac></mml:math> Heisenberg antiferromagnet on the shuriken lattice | Litcius