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Intracellular Synthesis of Indoles Enabled by Visible-Light Photocatalysis

Cinzia D’Avino, Sara Gutiérrez, Max J. Feldhaus, María Tomás‐Gamasa, José L. Mascareñas

2024Journal of the American Chemical Society35 citationsDOIOpen Access PDF

Abstract

Performing abiotic synthetic transformations in live cell environments represents a new, promising approach to interrogate and manipulate biology and to uncover new types of biomedical tools. We now found that photocatalytic bond-forming reactions can be added to the toolbox of bioorthogonal synthetic chemistry. Specifically, we demonstrate that exogenous styryl aryl azides can be converted into indoles inside living mammalian cells under photocatalytic conditions.

Topics & Concepts

ChemistryPhotocatalysisBioorthogonal chemistryIntracellularToolboxNanotechnologyArylCombinatorial chemistryCatalysisBiochemistryOrganic chemistryClick chemistryAlkylProgramming languageMaterials scienceComputer scienceClick Chemistry and ApplicationsRadical Photochemical ReactionsSynthesis and Catalytic Reactions