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Enhancing Self‐Powered Terahertz Photodetection with VSe<sub>2</sub> and Van Der Waals Heterostructure Integration via Photothermoelectric Effect

Mengjie Jiang, Xiaokai Pan, Kaixuan Zhang, Shijian Tian, Libo Zhang, Li Han, Yuan He, Xuyang Lv, Shiqi Lan, Huaizhong Xing, Lin Wang

2024Advanced Electronic Materials14 citationsDOIOpen Access PDF

Abstract

Abstract Owning unique optical and electronic properties, two dimensional (2D) materials have made remarkable strides in the field of photodetection applications. However, achieving highly sensitive and ultra‐broadband detection from microwave to terahertz (THz) range (0.02–0.54 THz) remains a significant challenge for photodetectors. This study presents a self‐powered THz photodetector based on VSe 2 and its van der Waals heterostructure. The photoresponse of the photodetector is primarily attributed to the photothermoelectric effect. At room temperature, the device exhibits lower noise equivalent power values of 21 pW Hz −1/2 at 0.28 THz. This work has achieved ultra‐broadband detection and demonstrated the potential for large‐area imaging, providing a new avenue for the application of THz technology in nondestructive testing and biometric identification fields.

Topics & Concepts

PhotodetectionTerahertz radiationPhotodetectorMaterials scienceOptoelectronicsvan der Waals forceHeterojunctionBroadbandGrapheneMicrowaveOpticsNanotechnologyPhysicsTelecommunicationsComputer scienceMoleculeQuantum mechanics2D Materials and ApplicationsTopological Materials and PhenomenaAdvanced Thermoelectric Materials and Devices
Enhancing Self‐Powered Terahertz Photodetection with VSe<sub>2</sub> and Van Der Waals Heterostructure Integration via Photothermoelectric Effect | Litcius