Litcius/Paper detail

Manipulating Weyl quasiparticles by orbital-selective photoexcitation in WTe2

Meng-Xue Guan, En Wang, Pei-Wei You, Jia-Tao Sun, Sheng Meng

2021Nature Communications44 citationsDOIOpen Access PDF

Abstract

Abstract Optical control of structural and electronic properties of Weyl semimetals allows development of switchable and dissipationless topological devices at the ultrafast scale. An unexpected orbital-selective photoexcitation in type-II Weyl material WTe 2 is reported under linearly polarized light (LPL), inducing striking transitions among several topologically-distinct phases mediated by effective electron-phonon couplings. The symmetry features of atomic orbitals comprising the Weyl bands result in asymmetric electronic transitions near the Weyl points, and in turn a switchable interlayer shear motion with respect to linear light polarization, when a near-infrared laser pulse is applied. Consequently, not only annihilation of Weyl quasiparticle pairs, but also increasing separation of Weyl points can be achieved, complementing existing experimental observations. In this work, we provide a new perspective on manipulating the Weyl node singularity and coherent control of electron and lattice quantum dynamics simultaneously.

Topics & Concepts

QuasiparticlePhotoexcitationPhysicsWeyl semimetalCondensed matter physicsQuantum mechanicsCoherent controlAtomic orbitalQuantumSingularityExcitationElectronDirac (video compression format)Ultrashort pulseLattice (music)AnnihilationFemtosecondSemimetalHigh harmonic generationMagneto opticalLorentz transformationQuantum dotStrongly correlated materialLaserElectronic band structureSymmetry (geometry)Topological Materials and Phenomena2D Materials and ApplicationsChemical and Physical Properties of Materials