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Chiral Brønsted acid-catalyzed asymmetric dearomative spirocyclization of alkynyl thioethers

Xin-Yang Fan, Jiacheng Li, Ji‐Jia Zhou, Bo Zhou, Long‐Wu Ye

2023Green Chemistry17 citationsDOI

Abstract

A chiral Brønsted acid-catalyzed asymmetric dearomative spirocyclization of alkynyl thioethers has been developed, leading to the green and atom-economical preparation of chiral sprio[4.5]decan-6-ones in good yields with high enatioselectivities.

Topics & Concepts

CatalysisBrønsted–Lowry acid–base theoryChemistryCombinatorial chemistryMedicinal chemistryOrganic chemistryCatalytic C–H Functionalization MethodsSulfur-Based Synthesis TechniquesOxidative Organic Chemistry Reactions
Chiral Brønsted acid-catalyzed asymmetric dearomative spirocyclization of alkynyl thioethers | Litcius