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Unraveling the relationship between the phenethylammonium-induced 2D phase on the perovskite surface and inverted wide bandgap perovskite solar cell performance

Xiaomin Huo, Silvia Mariotti, Yaoyao Li, Ting Yue Guo, Chenfeng Ding, Penghui Ji, Shuai Yuan, Tongtong Li, Ning Meng, Xiaomin Liu, Jiahao Zhang, Ilhem Nadia Rabehi, Yu Zhang, Suling Zhao, Hengyuan Wang, Dandan Song, Luis K. Ono, Zheng Xu, Yabing Qi

2024Energy & Environmental Science41 citationsDOI

Abstract

We studied the impact of phenethylammonium chloride on PIN-structured wide bandgap perovskite solar cells. Elimination of the 2D phase results in a champion efficiency of 20.61% and a V OC loss of only 410 mV with hysteresis-free J–V curves.

Topics & Concepts

Perovskite (structure)Materials scienceBand gapPerovskite solar cellSolar cellPhase (matter)OptoelectronicsCrystallographyPhysicsChemistryQuantum mechanicsPerovskite Materials and ApplicationsConducting polymers and applications