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Reversing a Platinum Micromotor by Introducing Platinum Oxide

Xianglong Lyu, Jingyuan Chen, Jiayu Liu, Yixin Peng, Shifang Duan, Xing Ma, Wei Wang

2022Angewandte Chemie International Edition18 citationsDOI

Abstract

Abstract Understanding and controlling the swimming direction of a synthetic nano‐ and micromotor holds fundamental and applied significance. Here, we focus on platinum‐containing Janus colloids that catalytically decompose H 2 O 2 into O 2 , an archetypical model of chemical micromotor. We discover that platinum oxides (primarily PtO) are produced on Pt films sputter‐coated in O 2 plasma, and PtO reverses the motor possibly by self‐electrophoresis. Using this knowledge, micromotors moving in either direction were fabricated by intentionally introducing or removing PtO. These findings challenge the conventional wisdom that a Pt micromotor is powered by Pt alone, and open up new avenues for controlling the swimming directions of a micro‐ and nanomachine.

Topics & Concepts

PlatinumReversingNanotechnologyJanusSputteringMaterials scienceOxideChemistryCatalysisThin filmComposite materialOrganic chemistryMetallurgyMicro and Nano RoboticsMolecular Communication and NanonetworksMicrofluidic and Bio-sensing Technologies
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