Litcius/Paper detail

Detecting and characterizing special nuclear material for nuclear nonproliferation applications

Sara A. Pozzi, Zhong He, Jesson Hutchinson, Igor Jovanovic, Ricardo Lopez, K. Ogren, J. Nattress, Daniel Shy, Shaun D. Clarke

2023Scientific Reports12 citationsDOIOpen Access PDF

Abstract

There is an urgent need for new, better instrumentation and techniques for detecting and characterizing special nuclear material (SNM), i.e., highly enriched uranium and plutonium. The development of improved instruments and techniques requires experiments performed with the SNM itself, which is of limited availability. This paper describes the findings of experiments performed at the National Criticality Experiments Research Center conducted using new instruments and techniques on unclassified, kg-quantity SNM objects. These experiments, performed in the framework of the Department of Energy, National Nuclear Security Administration Consortium for Monitoring, Technology, and Verification, focused on detecting, characterizing, and localizing SNM samples with masses ranging from 3.3 to 13.8 kg, including plutonium and highly enriched uranium using prototype detectors and techniques. The work demonstrates SNM detection and characterization using recently-developed prototype detection systems. Specifically, we present new results in passive detection and imaging of plutonium and uranium objects using gamma-ray and dual particle (fast neutron and gamma-ray) imaging. We also present a new analysis of the delayed neutron emissions during active interrogation of uranium using a neutron generator.

Topics & Concepts

PlutoniumEnriched uraniumNuclear engineeringUraniumNuclear materialNeutron generatorDepleted uraniumCriticalityNeutronInstrumentation (computer programming)Computer scienceEnvironmental scienceNeutron sourceNuclear physicsSystems engineeringPhysicsEngineeringOperating systemNuclear Physics and ApplicationsRadiation Detection and Scintillator TechnologiesNuclear reactor physics and engineering