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Low‐temperature synthesis one‐dimensional Ag <sub>2</sub> CO <sub>3</sub> /SnFe <sub>2</sub> O <sub>4</sub> <i>Z</i> ‐scheme with excellent visible‐light photoactivity

Xiaoli Su, Aihui Wang, Linyuan Xu, Wei Zhang, Fumin Guo, Dafeng Zhang, Xipeng Pu, Peiqing Cai

2023Journal of the American Ceramic Society28 citationsDOI

Abstract

Abstract In this study, Ag 2 CO 3 /SnFe 2 O 4 (Ag 2 CO 3 /SFO) photocatalyst was prepared by a simple hydrothermal‐ultrasonic method for the efficient degradation of ciprofloxacin and phenol. The SFO nanoparticles were attached on the surface of Ag 2 CO 3 rods synthesized by a low‐temperature precipitation method, resulting a unique 1D/0D morphology, which increased the number of active sites. Due to introduction of magnetic SFO, Ag 2 CO 3 /SFO exhibited excellent magnetic recovery performance. When the mass fraction of SFO was 5%, the degradation efficiency of composite photocatalyst was the highest, the degradation rate for ciprofloxacin was 6.5 and 1.5 times higher than pure SFO and Ag 2 CO 3 , respectively. The improved photoactivity of Ag 2 CO 3 /SFO should be attributed to the construction of heterojunction with tight interface, which boosts the separation and transfer of photoinduced electron and hole pairs. On the basis of experimental results, a possible Z ‐scheme photocatalytic mechanism was discussed. Additionally, the excellent photostability of Ag 2 CO 3 /SFO was proved by a cycle experiment.

Topics & Concepts

Materials sciencePhotocatalysisHydrothermal circulationHeterojunctionDegradation (telecommunications)Visible spectrumMass fractionPrecipitationChemical engineeringHigh-resolution transmission electron microscopyNuclear chemistryAnalytical Chemistry (journal)NanotechnologyChemistryComposite materialOptoelectronicsCatalysisTransmission electron microscopyOrganic chemistryComputer scienceMeteorologyPhysicsEngineeringTelecommunicationsAdvanced Photocatalysis TechniquesCopper-based nanomaterials and applicationsZnO doping and properties