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FeCl<sub>3</sub>-promoted regioselective synthesis of BODIPY dimers through oxidative aromatic homocoupling reactions

Zhengxin Kang, Qinghua Wu, Xing Guo, Long Wang, Yin Ye, Changjiang Yu, Hua Wang, Erhong Hao, Lijuan Jiao

2021Chemical Communications23 citationsDOI

Abstract

. This regioselective dimerization was achieved for BODIPYs substituted only in the 5-position with Cl or aryl groups. Further functionalization of the 5,5'-dichloride dimer gave the corresponding pyrrole or 4-(2-aminoethyl)morpholine disubstituted dimers 2f and 2g, respectively. While dimer 2f exhibited intense NIR absorption/emission maxima at 773/827 nm in toluene, dimer 2g showed favorable lysosome-targeting NIR fluorescence in living cells.

Topics & Concepts

BODIPYRegioselectivityOxidative phosphorylationChemistryOxidative coupling of methanePhotochemistryAbsorption (acoustics)Combinatorial chemistryFluorescenceOrganic chemistryMaterials scienceCatalysisBiochemistryQuantum mechanicsPhysicsComposite materialLuminescence and Fluorescent MaterialsNanoplatforms for cancer theranosticsMolecular Sensors and Ion Detection