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Cascade Cyclization of <i>N</i>-Cyanamide Alkenes for the Divergent Synthesis of Azido-, Nitro-, and Alkenyl-Containing Pyrroloquinazolinones

Bo Jiang, Cui Zhang, Tai‐Gang Fan, Yu‐Song Ran, Yun‐Tao Shen, Yuan Qu, Ya‐Min Li

2024Organic Letters24 citationsDOI

Abstract

-cyanamide alkenes have been developed for the divergent synthesis of pyrroloquinazolinones bearing azido, alkenyl, and nitro groups by controlling the reaction conditions. The reaction temperature and the loading of the base play important roles in the different reaction pathways. These reactions are characterized by wide functional group compatibility and mild conditions.

Topics & Concepts

ChemistryCascadeNitroCyanamideMedicinal chemistryCombinatorial chemistryOrganic chemistryStereochemistryChromatographyAlkylClick Chemistry and ApplicationsSynthesis and Biological EvaluationCyclopropane Reaction Mechanisms
Cascade Cyclization of <i>N</i>-Cyanamide Alkenes for the Divergent Synthesis of Azido-, Nitro-, and Alkenyl-Containing Pyrroloquinazolinones | Litcius