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Insights into the pH-Dependent Adsorption Behavior of Ionic Dyes on Phosphoric Acid-Activated Biochar

Wei Fang, Yuwei Zhu, Tongmin He, Shengpu Zhu, Tianhao Wang, Chunyi Yao, Chenlu Yu, Peipei Huang, Yan Li, Qiang Zhao, Weiguo Song

2022ACS Omega54 citationsDOIOpen Access PDF

Abstract

in the preparation of the adsorbent was investigated by a range of experiments and characterizations. The kinetic and isotherm experiments are also conducted to evaluate its dye adsorption behavior. According to the adsorption experiment results, PPC exhibits high saturated adsorption capacities for methyl orange (MO, 239.1 mg/g), rhodamine B (RhB, 2821.8 mg/g), methylene blue (MB, 580.5 mg/g), and crystal violate (CV, 396.6 mg/g) according to the Langmuir model. The maximum initial concentration of each dye solution for acquiring 90% removal efficiency is estimated to be 234.55 ppm (MO), 2943.8 ppm (RhB), 633.8 ppm (MB), and 423.6 ppm (CV) at 298 K with an adsorbent dosage of 1 g/L. The characterization results also indicate PPC has a complex synergetic mechanism for ionic dye adsorption behavior. This provides perspectives regarding PPC as a promising biochar adsorbent from biomass waste, which is probably useful for high-efficiency dye removal in water treatment.

Topics & Concepts

BiocharAdsorptionPhosphoric acidRhodamine BChemistryMethyl orangeMethylene blueLangmuir adsorption modelNuclear chemistryChemical engineeringOrganic chemistryPyrolysisPhotocatalysisCatalysisEngineeringAdsorption and biosorption for pollutant removalPhosphorus and nutrient managementNanomaterials for catalytic reactions