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Comprehensive Insight into <i>p</i>-Type Bi<sub>2</sub>Te<sub>3</sub>-Based Thermoelectrics near Room Temperature

Qing Shi, Juan Li, Xuanwei Zhao, Yiyuan Chen, Fujie Zhang, Yan Zhong, Ran Ang

2022ACS Applied Materials & Interfaces75 citationsDOI

Abstract

Bi2Te3 is a well-recognized material for its unique properties in diverse thermoelectric applications near room temperature. The considerable efforts on Bi2Te3-based alloys have been extremely extensive in recent years, and thus the latest breakthroughs in high-performance p-type (Bi, Sb)2Te3 alloys are comprehensively reviewed to further implement applications. Effective strategies to further improve the thermoelectric performance are summarized from the perspective of enhancing the power factor and minimizing the lattice thermal conductivity. Furthermore, the surface states of topological insulators are investigated to provide a possibility of advancing (Bi, Sb)2Te3 thermoelectrics. Finally, future challenges and outlooks are overviewed. This review will provide potential guidance toward designing and developing high-efficient Bi2Te3-based and other thermoelectrics.

Topics & Concepts

Materials scienceThermoelectric materialsEngineering physicsThermoelectric effectNanotechnologyOptoelectronicsThermal conductivityThermodynamicsComposite materialPhysicsAdvanced Thermoelectric Materials and DevicesTopological Materials and PhenomenaThermal Radiation and Cooling Technologies