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Van der Waals integration of high-κ perovskite oxides and two-dimensional semiconductors

Jian Yang, Kun Han, Ke Huang, Chen Ye, Wen Wen, Ruixue Zhu, Rui Zhu, Jun Xu, Ting Yu, Peng Gao, Qihua Xiong, Xiao Renshaw Wang

2022Nature Electronics213 citationsDOIOpen Access PDF

Abstract

Abstract Two-dimensional semiconductors can be used to build next-generation electronic devices with ultrascaled channel lengths. However, semiconductors need to be integrated with high-quality dielectrics—which are challenging to deposit. Here we show that single-crystal strontium titanate—a high- κ perovskite oxide—can be integrated with two-dimensional semiconductors using van der Waals forces. Strontium titanate thin films are grown on a sacrificial layer, lifted off and then transferred onto molybdenum disulfide and tungsten diselenide to make n-type and p-type transistors, respectively. The molybdenum disulfide transistors exhibit an on/off current ratio of 10 8 at a supply voltage of 1 V and a minimum subthreshold swing of 66 mV dec −1 . We also show that the devices can be used to create low-power complementary metal–oxide–semiconductor inverter circuits.

Topics & Concepts

SemiconductorMaterials sciencevan der Waals forceStrontium titanatePerovskite (structure)OptoelectronicsTransistorTungsten diselenideDielectricNanotechnologyVoltageElectrical engineeringChemistryCrystallographyTransition metalEngineeringMoleculeBiochemistryOrganic chemistryCatalysis2D Materials and ApplicationsPerovskite Materials and ApplicationsGraphene research and applications
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