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Elucidating the solution structure of the monomolecular <i>BCL2</i> RNA G-quadruplex: a new robust NMR assignment approach

Zenghui Wang, Carla Ferreira Rodrigues, Simon Jurt, Alicia Domínguez‐Martín, Silke Johannsen, Roland K. O. Sigel

2025Chemical Science6 citationsDOIOpen Access PDF

Abstract

proto-oncogene, one of the first natural monomolecular RNA G4 structures available to date. Comparative analysis with other RNA and DNA G4s reveals their notably compact and well-defined cores. Moreover, the sugar pucker geometries of the tetrad guanines are far less stringent than previously assumed, adeptly accommodating specific structural features. This contrasts with the canonical base pairing in RNA and DNA, in which the sugar pucker dictates the type of the double-helical structure. The strategy presented provides a direct path to uncovering G4 structural intricacies, advancing our grasp of their biological roles, and paving the way for RNA-targeted therapeutics.

Topics & Concepts

G-quadruplexRNAChemistryNucleic acid structureCombinatorial chemistryStereochemistryComputational biologyDNABiochemistryBiologyGeneRNA and protein synthesis mechanismsDNA and Nucleic Acid ChemistryRNA Interference and Gene Delivery