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Nicotinamide as Additive for Microcrystalline and Defect Passivated Perovskite Solar Cells with 21.7% Efficiency

Zhu Ma, Weiya Zhou, Dejun Huang, Qianyu Liu, Zheng Xiao, Huifeng Jiang, Zhiqing Yang, Wenfeng Zhang, Yuelong Huang

2020ACS Applied Materials & Interfaces90 citationsDOI

Abstract

and/or FAI: MABr: MACl precursor solution to obtain NTM modified perovskite films. It has been found that the NTM in the perovskite film can well passivate surface and GBs defects, control the film morphology and enhance the crystallinity via its interaction with a lone pair of electrons in nitrogen. In the presence of the NTM additive, we obtained enlarged perovskite crystal grain about 3.6 μm and a champion planar perovskite solar cell with efficiency of 21.72% and negligible hysteresis. Our findings provide an effective route for crystal growth and defect passivation to bring further increases on both efficiency and stability of perovskite solar cells.

Topics & Concepts

PassivationMaterials sciencePerovskite (structure)CrystallinityGrain boundaryPerovskite solar cellEnergy conversion efficiencyChemical engineeringCrystal (programming language)HysteresisNanotechnologyOptoelectronicsLayer (electronics)Composite materialMicrostructureEngineeringComputer sciencePhysicsProgramming languageQuantum mechanicsPerovskite Materials and ApplicationsChalcogenide Semiconductor Thin FilmsQuantum Dots Synthesis And Properties
Nicotinamide as Additive for Microcrystalline and Defect Passivated Perovskite Solar Cells with 21.7% Efficiency | Litcius