Litcius/Paper detail

Exciton-activated effective phonon magnetic moment in monolayer <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mi>MoS</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math>

Chunli Tang, Gaihua Ye, Cynthia Nnokwe, Mengqi Fang, Li Xiang, Masoud Mahjouri‐Samani, Dmitry Smirnov, Eui‐Hyeok Yang, Tingting Wang, Lifa Zhang, Rui He, Wencan Jin

2024Physical review. B./Physical review. B11 citationsDOIOpen Access PDF

Abstract

Chiral phonons are lattice vibration modes in which the atomic circular motions produce nonzero angular momentum. In monolayer MoS${}_{2}$, the authors demonstrate here a chiral phonon mode at ~270 cm${}^{\ensuremath{-}1}$ that is activated by resonant excitation of the bright exciton. Under an out-of-plane magnetic field, this mode exhibits large Zeeman splitting, which corresponds to an effective magnetic moment of ~2.5 \ensuremath{\mu}${}_{B}$. This study will stimulate research on the effective magnetic moments that emerge from the interplay between chiral phonons and the valley degree of freedom.

Topics & Concepts

MonolayerExcitonPhononMagnetic momentCondensed matter physicsMoment (physics)PhysicsMaterials scienceQuantum mechanicsNanotechnologyOrganic and Molecular Conductors Research2D Materials and ApplicationsSpectroscopy and Quantum Chemical Studies