Litcius/Paper detail

Effects of surface roughness on CMAS corrosion behavior for thermal barrier coating applications

Lei Guo, Guang Li, Zhilin Gan

2021Journal of Advanced Ceramics107 citationsDOIOpen Access PDF

Abstract

Abstract Calcium-magnesium-alumina-silicate (CMAS) corrosion is an important cause for thermal barrier coating (TBC) failure, which has attracted increased attentions. In this study, some thermal barrier coating (TBC) materials including YSZ (yttria partially stabilized zirconia), GdPO 4 , and LaPO 4 were prepared into bulks, and the effects of their surface roughness on wettability and spreading characteristics of molten CMAS were investigated. As-fabricated and polished bulks with different surface roughness were exposed to CMAS corrosion at 1250 °C for 1 and 4 h, following by macro and micro observations. Results revealed that compared with the as-fabricated bulks, molten CMAS on the polished samples had lower wettability and a smaller spreading area, mainly attributable to the reduced capillary force to drive the melt spreading. Meanwhile, GdPO 4 and LaPO 4 bulks exhibited lower CMAS wettability than YSZ bulk. It is thus considered that reducing the surface roughness is beneficial to CMAS corrosion resistance of TBCs.

Topics & Concepts

Materials scienceThermal barrier coatingWettingCoatingCorrosionYttria-stabilized zirconiaSurface roughnessCubic zirconiaSurface finishMetallurgyContact angleComposite materialInconelCeramicAlloyHigh-Temperature Coating BehaviorsAdvanced materials and compositesNuclear Materials and Properties