Litcius/Paper detail

Characterization of N‐doped carbon quantum dots synthesized by DBD‐based cold atmospheric pressure plasma jet

Mina Mohammadzaheri, Vahid Siahpoush, Asghar Asgari

2022Plasma Processes and Polymers16 citationsDOI

Abstract

Abstract This study develops a new approach for the synthesis of fluorescent N‐doped carbon quantum dots (CQDs), using cold atmospheric pressure plasma jet. Herein, the CQDs were synthesized with two plasma exposure times of 30 and 60 min. The UV‐Vis absorption spectrum confirms the existence of carbonic core and surface functional groups. The Fourier transform infrared spectrum shows that carbonyl groups and amide groups exist on the surface of CQDs. Depending on the plasma exposure time, the mean average sizes of CQDs are 3.63 and 5.45 nm with strong photoluminescence emission. Generally, our results indicated that using different mechanisms for plasma discharge, lead to different physical and chemical properties of produced plasma and consequently of synthesized CQDs. The synthesized N‐doped CQDs exhibited strong fluorescence and higher quantum yield compared to previous reports.

Topics & Concepts

PhotoluminescenceQuantum yieldFourier transform infrared spectroscopyAtmospheric pressureFluorescenceAtmospheric-pressure plasmaMaterials sciencePlasmaDopingInfraredAnalytical Chemistry (journal)Carbon fibersAbsorption (acoustics)Jet (fluid)PhotochemistryChemistryChemical engineeringOptoelectronicsOrganic chemistryOpticsComposite numberComposite materialThermodynamicsPhysicsQuantum mechanicsEngineeringOceanographyGeologyCarbon and Quantum Dots ApplicationsNanocluster Synthesis and ApplicationsLuminescence and Fluorescent Materials