Litcius/Paper detail

Enhancing the energy storage performances of metal–organic frameworks by controlling microstructure

Jamie W. Gittins, Chloe J. Balhatchet, Simon M. Fairclough, Alexander C. Forse

2022Chemical Science66 citationsDOIOpen Access PDF

Abstract

(HHTP = 2,3,6,7,10,11-hexahydroxytriphenylene) with distinct microstructures. Supercapacitors assembled with these samples conclusively demonstrate that sample microstructure and particle morphology have a significant impact on the energy storage performances of MOFs. Samples with 'flake-like' particles, with a pore network comprised of many short pores, display superior capacitive performances than samples with either 'rod-like' or strongly agglomerated particles. The results of this study provide a target microstructure for conductive MOFs for energy storage applications.

Topics & Concepts

Metal-organic frameworkMicrostructureEnergy storageEnergy (signal processing)Materials scienceNanotechnologyProcess engineeringMetallurgyChemistryOrganic chemistryEngineeringPhysicsThermodynamicsQuantum mechanicsAdsorptionPower (physics)Supercapacitor Materials and FabricationMetal-Organic Frameworks: Synthesis and ApplicationsAdvanced Battery Technologies Research