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Combined Effects of Anion Substitution and Nanoconfinement on the Ionic Conductivity of Li-Based Complex Hydrides

Roman Zettl, Laura M. de Kort, Maria Gombotz, Martin Wilkening, Petra E. de Jongh, Peter Ngene

2020The Journal of Physical Chemistry C49 citationsDOIOpen Access PDF

Abstract

, concomitant with a lowered activation energy of 0.44 eV for Li-ion transport. Our work demonstrates that a combination of partial ion substitution and nanoconfinement is an effective strategy to boost the ionic conductivity of complex hydrides. The strategy could be applicable to other classes of solid-state electrolytes.

Topics & Concepts

ElectrolyteIonic conductivityLithium (medication)IonIonic bondingMaterials scienceConductivityFast ion conductorInorganic chemistryWork (physics)Chemical engineeringChemistryPhysical chemistryThermodynamicsElectrodeOrganic chemistryEngineeringPhysicsMedicineEndocrinologyHydrogen Storage and MaterialsAdvanced Battery Materials and TechnologiesAmmonia Synthesis and Nitrogen Reduction
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