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Structural basis of K11/K48-branched ubiquitin chain recognition by the human 26S proteasome

Piotr Drączkowski, Szu-Ni Chen, Ting Chen, Yong‐Sheng Wang, Hsin-An Shih, Jessica Y. C. Huang, Ming-Chieh Tsai, Shu‐Yu Lin, Steven Lin, Rosa Viner, Yuan‐Chih Chang, Kuen‐Phon Wu, Shang‐Te Danny Hsu

2025Nature Communications11 citationsDOIOpen Access PDF

Abstract

Beyond the canonical K48-linked homotypic polyubiquitination for proteasome-targeted proteolysis, K11/K48-branched ubiquitin (Ub) chains are involved in fast-tracking protein turnover during cell cycle progression and proteotoxic stress. Here, we report cryo-EM structures of human 26S proteasome in a complex with a K11/K48-branched Ub chain. The structures revealed a multivalent substrate recognition mechanism involving a hitherto unknown K11-linked Ub binding site at the groove formed by RPN2 and RPN10 in addition to the canonical K48-linkage binding site formed by RPN10 and RPT4/5 coiled-coil. Additionally, RPN2 recognizes an alternating K11-K48-linkage through a conserved motif similar to the K48-specific T1 binding site of RPN1. The insights gleaned from these structures explain the molecular mechanism underlying the recognition of the K11/K48-branched Ub as a priority signal in the ubiquitin-mediated proteasomal degradation.

Topics & Concepts

UbiquitinProteasomeCell biologyChemistryUbiquitin-Protein LigasesPlasma protein bindingUbiquitin ligaseBinding siteMechanism (biology)BiochemistryUbiquitinsProtein–protein interactionProtein structureSubstrate specificityBiophysicsThreading (protein sequence)Peptide sequenceMolecular recognitionComputational biologySubstrate (aquarium)BiologyDeubiquitinating enzymeSequence homologyCellUbiquitin-conjugating enzymeCell cycle progressionLysineProtein degradationConserved sequenceUbiquitin and proteasome pathwaysRNA modifications and cancerPeptidase Inhibition and Analysis
Structural basis of K11/K48-branched ubiquitin chain recognition by the human 26S proteasome | Litcius