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Fluid Viscoelasticity Triggers Fast Transitions of a Brownian Particle in a Double Well Optical Potential

Brandon R. Ferrer, Juan Ruben Gomez-Solano, Alejandro V. Arzola

2021Physical Review Letters46 citationsDOIOpen Access PDF

Abstract

Thermally activated transitions are ubiquitous in nature, occurring in complex environments which are typically conceived as ideal viscous fluids. We report the first direct observations of a Brownian bead transiting between the wells of a bistable optical potential in a viscoelastic fluid with a single long relaxation time. We precisely characterize both the potential and the fluid, thus enabling a neat comparison between our experimental results and a theoretical model based on the generalized Langevin equation. Our findings reveal a drastic amplification of the transition rates compared to those in a Newtonian fluid, stemming from the relaxation of the fluid during the particle crossing events.

Topics & Concepts

Brownian motionViscoelasticityRelaxation (psychology)Langevin equationComplex fluidBrownian dynamicsNewtonian fluidPhysicsParticle (ecology)BistabilitySmoothed-particle hydrodynamicsRheologyOptical tweezersMechanicsStatistical physicsClassical mechanicsThermodynamicsOpticsQuantum mechanicsGeologySocial psychologyOceanographyPsychologystochastic dynamics and bifurcationSpectroscopy and Quantum Chemical StudiesAdvanced Thermodynamics and Statistical Mechanics
Fluid Viscoelasticity Triggers Fast Transitions of a Brownian Particle in a Double Well Optical Potential | Litcius