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Out-of-plane bond-order phase, superconductivity, and their competition in the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mi>t</mml:mi> </mml:math> - <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi>J</mml:mi> <mml:mo>∥</mml:mo> </mml:msub> <mml:mtext>−</mml:mtext> <mml:msub> <mml:mi>J</mml:mi> <mml:mo>⊥</mml:mo> </mml:msub> </mml:math> model: Possible implications for bilayer nickelates

Matías Bejas, Xianxin Wu, Debmalya Chakraborty, Andreas P. Schnyder, A. Greco

2025Physical review. B./Physical review. B9 citationsDOI

Abstract

Almost four decades of intense research have been invested to study the physics of high-${T}_{c}$ cuprate superconductors. The recent discovery of high-${T}_{c}$ superconductivity in pressurized bilayer nickelates and its potential similarities with cuprate superconductors may open a new window to understand this long-standing problem. We have studied the proposed bilayer $t\text{\ensuremath{-}}{J}_{\ensuremath{\parallel}}\text{\ensuremath{-}}{J}_{\ensuremath{\perp}}$ model [where ${J}_{\ensuremath{\parallel}}$ (${J}_{\ensuremath{\perp}}$) is the in-plane (out-of-plane) magnetic exchange] in a large-$N$ approach on the basis of the path integral representation for Hubbard operators, which allows to obtain results at mean-field and beyond mean-field level. We find that ${J}_{\ensuremath{\perp}}$ is a candidate for triggering high superconducting ${T}_{c}$ values at quarter filling (hole doping $\ensuremath{\delta}=0.5$) of the ${d}_{{x}^{2}\ensuremath{-}{y}^{2}}$ orbitals. Beyond mean-field level, we find a new phase, an out-of-plane bond-order phase (z-BOP), triggered also by ${J}_{\ensuremath{\perp}}$. z-BOP develops below a critical temperature which decreases with increasing doping and vanishes at a quantum critical point below quarter filling. The occurrence of this phase and its competition with superconductivity leads to a superconducting dome-shaped behavior as a function of doping and as a function of ${J}_{\ensuremath{\perp}}$. Qualitative comparisons with the physics of cuprates and the recent literature on the new pressurized nickelates are given along the paper.

Topics & Concepts

Order (exchange)Plane (geometry)MathematicsCombinatoricsDiscrete mathematicsGeometryFinanceEconomicsPhysics of Superconductivity and MagnetismAdvanced Condensed Matter PhysicsOrganic and Molecular Conductors Research
Out-of-plane bond-order phase, superconductivity, and their competition in the <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:mi>t</mml:mi> </mml:math> - <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msub> <mml:mi>J</mml:mi> <mml:mo>∥</mml:mo> </mml:msub> <mml:mtext>−</mml:mtext> <mml:msub> <mml:mi>J</mml:mi> <mml:mo>⊥</mml:mo> </mml:msub> </mml:math> model: Possible implications for bilayer nickelates | Litcius