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Construction of Collagen Methacrylamide Microspheres to Modify Nonwoven Polyamide Fibers Based on Click Chemistry

Na Xu, Yanmei Xing, Xuechuan Wang

2021ACS Applied Polymer Materials14 citationsDOI

Abstract

Using waste leather collagen, collagen microspheres with “–CH═CH2” (CMAs) were prepared using the emulsification cross-linking method and then incorporated into a nonwoven polyamide fiber material with the “thiol–ene” click chemistry method to obtain modified nonwoven polyamide fibers (PA-CMAs). Experiments showed that for a CMA concentration of 6 wt %, initiator concentration of 0.008 wt %, and irradiation time of 5 h, the grafting rate can reach 25.83%. Scanning electron microscope (SEM) and X-ray photoelectron spectrometer (XPS) are used to confirm the successful grafting of CMAs onto nonwoven PA materials. The stability and fastness test was used to show that PA-CMAs have good stability with acid, alkali, organic solvent resistance, and rubbing resistance. The contrast test indicated that the moisture absorption and permeability of PA-CMAs were better than those of nonwoven polyamide/polyurethane (PA/PU), which is a synthetic leather-based material considered as one of the mainstream products. In addition, PA-CMAs maintained the original softness and elastoplasticity of PA.

Topics & Concepts

PolyamideMaterials sciencePolyurethaneGraftingChemical engineeringThermosetting polymerScanning electron microscopePolymer chemistryComposite materialPolymerEngineeringCollagen: Extraction and CharacterizationBone Tissue Engineering MaterialsSilk-based biomaterials and applications
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