Litcius/Paper detail

Benchtop access to anhydrous actinide N-donor coordination complexes using ionic liquids

Steven P. Kelley, Volodymyr Smetana, Stephen D. Emerson, Anja‐Verena Mudring, Robin D. Rogers

2020Chemical Communications17 citationsDOIOpen Access PDF

Abstract

By dehydrating actinide salts with an ionic liquid containing a common anion and subsequent reaction with N-heterocyclic ligands, we challenge the concept that actinides prefer O- over N-donors; rather the acidic hydrogen atoms of protic solvents hinder the formation of more elusive f-element N-donor coordination complexes.

Topics & Concepts

ActinideAnhydrousIonic liquidChemistryCoordination complexIonic bondingIonInorganic chemistryOrganic chemistryCatalysisMetalRadioactive element chemistry and processingIonic liquids properties and applicationsCoordination Chemistry and Organometallics