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Arene dearomatization through a catalytic N-centered radical cascade reaction

Rory C. McAtee, Efrey A. Noten, Corey R. J. Stephenson

2020Nature Communications114 citationsDOIOpen Access PDF

Abstract

Arene dearomatization reactions are an important class of synthetic technologies for the rapid assembly of unique chemical architectures. Herein, we report a catalytic protocol to initiate a carboamination/dearomatization cascade that proceeds through transient sulfonamidyl radical intermediates formed from native sulfonamide N-H bonds leading to 1,4-cyclohexadiene-fused sultams. Importantly, this work demonstrates a facile approach to employ two-dimensional aromatic compounds as modular building blocks to generate richly substituted, three-dimensional compounds. These reactions occur at room temperature under visible light irradiation and are catalyzed by the combination of an iridium(III) photocatalyst and a dialkyl phosphate base. Reaction optimization, substrate scope, mechanistic features, and synthetic applications of this transformation are presented.

Topics & Concepts

Combinatorial chemistryCatalysisCascade reactionChemistryIridiumSubstrate (aquarium)CascadePhotoredox catalysisPhotocatalysisOrganic chemistryOceanographyChromatographyGeologySulfur-Based Synthesis TechniquesRadical Photochemical ReactionsCatalytic C–H Functionalization Methods