Litcius/Paper detail

Ring-amplified shock tube for variable-gain, multi-wavelength absorption spectroscopy

Christopher L. Strand, Devin Merrell, Alexis Thoeny, Jesse W. Streicher, Ronald Hanson

2025Optics Express8 citationsDOIOpen Access PDF

Abstract

A ring-amplified shock tube (RAST) is presented as a new facility design for high-sensitivity laser absorption spectroscopy (LAS) in shock-heated experiments. By integrating a confocal, segmented circular multi-pass cell (SC-MPC) into the test section, the RAST decouples optical pathlength from tube diameter, enabling multi-pass absorption spectroscopy (MPAS) with selectable pathlengths ranging from 0.15 m to 11 m using single-entry alignment. Pathlengths well in excess of 11 m are possible by combining multiple cavity modes through re-entrant beam alignment. Design details of the constructed facility are provided and complemented with a generalized analytical framework for calculating the modes and beam pattern characteristics of SC-MPC optical cavities. A high-temperature air chemistry experiment targeting O 2 (X 3 Σ) at 221.6 nm, O(3s 5 S 2 o ) at 777 nm, N 2 (A 3 Σ) at 868 nm, and N(3s 4 P 5/2 ) at 868 nm demonstrates multi-wavelength, variable-gain measurements of absorption transitions previously undetectable at the target conditions. Results confirm robust beam alignment, low cavity noise, and minimal emission interference. The RAST provides substantial improvements in sensitivity and diagnostic flexibility for kinetics and spectroscopy applications.

Topics & Concepts

OpticsSpectroscopyMaterials scienceShock tubeAbsorption (acoustics)Absorption spectroscopyBeam (structure)Attenuation coefficientTube (container)Tunable diode laser absorption spectroscopyLaserSensitivity (control systems)Shock (circulatory)Cavity ring-down spectroscopyOptical cavityFlexibility (engineering)Raman spectroscopyOptical fiberSpectral lineTime-resolved spectroscopyStimulated emissionEmission spectrumSpectroscopy and Laser ApplicationsAtomic and Molecular PhysicsLaser-Matter Interactions and Applications